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Response of insulator surfaces to slow highly charged ions

Response of insulator surfaces to slow highly charged ions

Friedrich Aumayr (ORCID: 0000-0002-9788-0934)
  • Grant DOI 10.55776/P17449
  • Funding program Principal Investigator Projects
  • Status ended
  • Start September 1, 2004
  • End August 31, 2008
  • Funding amount € 247,422
  • Project website

Disciplines

Physics, Astronomy (100%)

Keywords

    Image Charge Acceleration, Electron Emission, Highly Charged Ions, Ion Surface Collisions, Hole Mobility, Dielectric Response Of Insulators

Abstract Final report

The interaction of slow highly charged ions (HCI) with solid surfaces results in the formation of "hollow atoms", an exotic atomic state far from equilibrium. Whereas electronic transitions, which eventually restore the equilibrium could largely be identified for metal surfaces in experimental and theoretical studies during the last decade, similar processes at insulator surfaces are much less understood. The main differences as compared to HCI - metal interactions are (i) the different dielectric response of insulating surfaces (modified image charge acceleration, reduced hole mobility, etc.), (ii) local charging-up of the surface (leading to a partial repulsion of the projectile by positive hole charges on the surface), and (iii) the wide electronic band gap (altering transfer, excitation and emission of electrons). In order to study the response of an insulator surface to the strong perturbation introduced by a slowly approaching highly charged ion, specifically designed experiments will be carried out at TU Wien (with moderately charged HCI in charge states q < 20), and at Max Planck Institute of Nuclear Physics in Heidelberg/Germany for ions in much higher charge states q = 60). In particular, we will investigate electron emission, image charge attraction and electronic excitation of different insulator target surfaces. Accompanying simulations at the Institute for Theoretical Physics TU Wien will support the interpretation of the obtained experimental results.

The interaction of slow highly charged ions (HCI) with solid surfaces results in the formation of "hollow atoms", an exotic atomic state far from equilibrium. Whereas electronic transitions, which eventually restore the equilibrium could largely be identified for metal surfaces in experimental and theoretical studies during the last decade, similar processes at insulator surfaces are much less understood. The main differences as compared to HCI - metal interactions are 1. the different dielectric response of insulating surfaces (modified image charge acceleration, reduced hole mobility, etc.), 2. local charging-up of the surface (leading to a partial repulsion of the projectile by positive hole charges on the surface), and 3. the wide electronic band gap (altering transfer, excitation and emission of electrons). In order to study the response of an insulator surface to the strong perturbation introduced by a slowly approaching highly charged ion, specifically designed experiments will be carried out at TU Wien (with moderately charged HCI in charge states q < 20), and at Max Planck Institute of Nuclear Physics in Heidelberg/Germany for ions in much higher charge states q = 60). In particular, we will investigate electron emission, image charge attraction and electronic excitation of different insulator target surfaces. Accompanying simulations at the Institute for Theoretical Physics TU Wien will support the interpretation of the obtained experimental results.

Research institution(s)
  • Technische Universität Wien - 100%
International project participants
  • Joachim Ullrich, Max-Planck-Institut - Germany

Research Output

  • 740 Citations
  • 19 Publications
Publications
  • 2012
    Title Charging dynamics in electron transmission through Al2O3 capillaries
    DOI 10.1016/j.nimb.2011.10.034
    Type Journal Article
    Author Milosavljevic A
    Journal Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and
    Pages 190-193
  • 2009
    Title Vanishing gap in LiF for electronic excitations by slow antiprotons
    DOI 10.1103/physrevb.79.125107
    Type Journal Article
    Author Solleder B
    Journal Physical Review B
    Pages 125107
    Link Publication
  • 2009
    Title Simulation of attosecond streaking of electrons emitted from a tungsten surface
    DOI 10.1103/physreva.79.062901
    Type Journal Article
    Author Lemell C
    Journal Physical Review A
    Pages 062901
    Link Publication
  • 2009
    Title Electronic stopping of low-energy H and He in Cu and Au investigated by time-of-flight low-energy ion scattering
    DOI 10.1103/physrevb.80.205105
    Type Journal Article
    Author Markin S
    Journal Physical Review B
    Pages 205105
  • 2009
    Title Electron Guiding through Insulating Nanocapillaries
    DOI 10.1103/physrevlett.102.163201
    Type Journal Article
    Author Schiessl K
    Journal Physical Review Letters
    Pages 163201
  • 2008
    Title Creation of Nanohillocks on CaF2 Surfaces by Single Slow Highly Charged Ions
    DOI 10.1103/physrevlett.100.237601
    Type Journal Article
    Author El-Said A
    Journal Physical Review Letters
    Pages 237601
  • 2008
    Title Nano-sized surface modifications induced by the impact of slow highly charged ions – A first review
    DOI 10.1016/j.nimb.2008.03.106
    Type Journal Article
    Author Aumayr F
    Journal Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and
    Pages 2729-2735
  • 2008
    Title Excitation energy and pair correlation function of trions near an LiF surface
    DOI 10.1103/physrevb.78.155432
    Type Journal Article
    Author Solleder B
    Journal Physical Review B
    Pages 155432
    Link Publication
  • 2008
    Title Electronic interaction of very slow light ions in Au: Electronic stopping and electron emission
    DOI 10.1103/physrevb.78.195122
    Type Journal Article
    Author Markin S
    Journal Physical Review B
    Pages 195122
  • 2007
    Title Spin-dependent low-energy electron transport in metals
    DOI 10.1103/physrevb.76.075115
    Type Journal Article
    Author Solleder B
    Journal Physical Review B
    Pages 075115
  • 2007
    Title Creation of surface nanostructures by irradiation with slow, highly charged ions
    DOI 10.1080/10420150701470803
    Type Journal Article
    Author El-Said A
    Journal Radiation Effects and Defects in Solids
    Pages 467-472
  • 2007
    Title On the nano-hillock formation induced by slow highly charged ions on insulator surfaces
    DOI 10.1016/j.sse.2007.06.016
    Type Journal Article
    Author Lemell C
    Journal Solid-State Electronics
    Pages 1398-1404
  • 2007
    Title Interaction of slow multicharged ions with surfaces
    DOI 10.1016/j.radphyschem.2005.09.024
    Type Journal Article
    Author Lemell C
    Journal Radiation Physics and Chemistry
    Pages 412-417
  • 2007
    Title Potential energy threshold for nano-hillock formation by impact of slow highly charged ions on a CaF2(111) surface
    DOI 10.1016/j.nimb.2006.12.142
    Type Journal Article
    Author El-Said A
    Journal Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and
    Pages 167-171
    Link Publication
  • 2007
    Title Electron emission by N6+ ions scattered at a magnetized iron surface
    DOI 10.1016/j.nimb.2006.12.100
    Type Journal Article
    Author Solleder B
    Journal Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and
    Pages 130-133
  • 2007
    Title Surface nanostructures induced by slow highly charged ions on CaF2 single crystals
    DOI 10.1016/j.nimb.2006.12.140
    Type Journal Article
    Author El-Said A
    Journal Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and
    Pages 346-349
  • 2007
    Title Highly charged ion-induced potential electron emission from clean Au(111): Dependence on the projectile angle of incidence
    DOI 10.1016/j.nimb.2006.12.102
    Type Journal Article
    Author Meissl W
    Journal Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and
    Pages 520-523
  • 2010
    Title Interaction potentials for fast atoms in front of Al surfaces probed by rainbow scattering
    DOI 10.1103/physrevb.82.125453
    Type Journal Article
    Author Tiwald P
    Journal Physical Review B
    Pages 125453
  • 2006
    Title Novel method for unambiguous ion identification in mixed ion beams extracted from an electron beam ion trap
    DOI 10.1063/1.2238856
    Type Journal Article
    Author Meissl W
    Journal Review of Scientific Instruments
    Pages 093303
    Link Publication

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