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Spin - Orbital Angular Momentum Entanglement with Neutrons

Stephan Sponar (ORCID: 0000-0002-6568-6045)
  • Grant DOI 10.55776/P34239
  • Funding program Principal Investigator Projects
  • Status ended
  • Start January 1, 2021
  • End December 31, 2025
  • Funding amount € 399,875
  • Project website

Disciplines

Physics, Astronomy (100%)

Keywords

  • Neutron,
  • Spin,
  • Angular Momentum,
  • Spin-Echo,
  • Interferometry,
  • Polarimetry
Abstract Final report

It has been long known that Orbital Angular Momentum (OAM) of bound massive particles and free photons is quantized. However, in recent years stable OAM has also been observed in free massive particles, namely electrons. Even more recently it was demonstrated that OAM states can be prepared in free thermal neutrons using a spiral phase plate. This type of OAM is characterized as extrinsic OAM, which refers to the fact that each neutron in the beam has the same OAM with respect to the optical axis of the beam, but has a different intrinsic OAM, that is to say OAM with respect to their respective momentum vector. Thus new methods for generating OAM in neutrons were developed theoretically. It is predicted that a magnetic quadrupole can be used to create neutron OAM, entangled to the neutron spin (spin-orbit states). In addition to this existing theoretically method, we propose to apply static homogeneous electric field to generate OAM. Field polarization along the direction of particle propagation induces longitudinal spin orbit states, while a transversely polarized electric field generates transverse spin orbit states. Transversal OAM, induced by static electric fields, has not yet been observed in massive free particles. To sum up, the aim of the project is to prepare and identify longitudinal and transversal entangled spin orbit states with neutrons.

It has been long known that Orbital Angular Momentum (OAM) of bound massive particles and free photons is quantized. However, in recent years stable OAM has also been observed in free massive particles, namely electrons. Even more recently it was demonstrated that OAM states can be prepared in free thermal neutrons using a spiral phase plate. This type of OAM is characterized as extrinsic OAM, which refers to the fact that each neutron in the beam has the same OAM with respect to the optical axis of the beam, but has a different intrinsic OAM, that is to say OAM with respect to their respective momentum vector. Thus, new methods for generating OAM in neutrons were developed theoretically. It is predicted that a magnetic quadrupole can be used to create neutron OAM, entangled to the neutron spin (spin-orbit states). In addition to this existing theoretically method, we propose to apply static homogeneous electric field to generate OAM. Field polarization along the direction of particle propagation induces longitudinal spin orbit states, while a transversely polarized electric field generates transverse spin orbit states. Transversal OAM, induced by static electric fields, has not yet been observed in massive free particles. Within the framework of this projected we able to demonstrate OAM generation via Schwinger scattering in perfect Quartz, utilizing the internal electric fields of the asymmetric crystal. Furthermore, we generalize magnetic methods which employ coherent averaging and apply this to neutron interferometry. Two aluminium prisms are inserted into a nested loop interferometer to generate a phase vortex lattice with significant extrinsic OAM. Moreover, we could show the applicability of our mode entangled interferometer at Atominstitut Tu Wien to generaate OAM via a procedure called coherent averaging; a new spin echo interferometry tool, which uses incomplete recombination of the two path states to generate composite wavefunctions with special structure. In particular we show that this method produces neutron wavefunctions that exist in a superposition of two quantum mechanical OAM modes, l = 1. Finally, a coupling between Earth's rotation and orbital angular momentum (OAM), known as the Sagnac effect, is observed in entangled neutrons produced using a spin-echo interferometer. After correction for instrument systematics the measured coupling is within 5% of theory, with an uncertainty of 7.2%. This demonstrates the feasibility of using the Sagnac effect to definitively measure neutron OAM and paves the way towards a future observation of the quantum Sagnac effect.

Research institution(s)
  • Technische Universität Wien - 100%
International project participants
  • Jeroen Plomp, Delft University of Technology - Netherlands
  • Michel Thijs, Delft University of Technology - Netherlands
  • W. Michael Snow, Indiana University Bloomington - USA

Research Output

  • 77 Citations
  • 15 Publications
Publications
  • 2025
    Title Generation and Detection of Neutron Orbital Angular Momentum
    Type PhD Thesis
    Author Niels Geerits
  • 2024
    Title CANISIUS The Austrian Neutron Spin Echo Interferometer
    DOI 10.48550/arxiv.2408.06216
    Type Preprint
    Author Geerits N
    Link Publication
  • 2024
    Title Covariant correlation-disturbance and its experimental realization with spin-1/2 particles
    DOI 10.48550/arxiv.2410.21918
    Type Preprint
    Author Asadian A
    Link Publication
  • 2024
    Title Violation of a Leggett-Garg Inequality Using Ideal Negative Measurements in Neutron Interferometry.
    DOI 10.1103/physrevlett.132.260201
    Type Journal Article
    Author Kreuzgruber E
    Journal Physical review letters
    Pages 260201
  • 2023
    Title Phase vortex lattices in neutron interferometry
    DOI 10.1038/s42005-023-01318-6
    Type Journal Article
    Author Geerits N
    Journal Communications Physics
    Pages 209
    Link Publication
  • 2023
    Title Violation of a Leggett-Garg inequality using ideal negative measurements in neutron interferometry
    DOI 10.48550/arxiv.2307.04409
    Type Preprint
    Author Kreuzgruber E
  • 2023
    Title Neutron Interferometer Experiments Studying Fundamental Features of Quantum Mechanics
    DOI 10.3390/atoms11060098
    Type Journal Article
    Author Danner A
    Journal Atoms
    Pages 98
    Link Publication
  • 2025
    Title Measuring the angular momentum of a neutron using Earth's rotation
    DOI 10.1103/physrevresearch.7.013046
    Type Journal Article
    Author Geerits N
    Journal Physical Review Research
    Pages 013046
    Link Publication
  • 2025
    Title Tight qubit uncertainty relations studied through weak values in neutron interferometry
    DOI 10.1103/pthn-81pm
    Type Journal Article
    Author Dvorak A
    Journal Physical Review Research
    Pages 043334
    Link Publication
  • 2021
    Title Neutron-state entanglement with overlapping paths
    DOI 10.1103/physrevresearch.3.023227
    Type Journal Article
    Author Kuhn S
    Journal Physical Review Research
    Pages 023227
    Link Publication
  • 2021
    Title Twisting neutral particles with electric fields
    DOI 10.1103/physreva.103.022205
    Type Journal Article
    Author Geerits N
    Journal Physical Review A
    Pages 022205
    Link Publication
  • 2022
    Title Quantifying the presence of a neutron in the paths of an interferometer
    DOI 10.48550/arxiv.2202.00272
    Type Preprint
    Author Lemmel H
  • 2022
    Title Quantifying the presence of a neutron in the paths of an interferometer
    DOI 10.1103/physrevresearch.4.023075
    Type Journal Article
    Author Lemmel H
    Journal Physical Review Research
    Pages 023075
    Link Publication
  • 2022
    Title Phase Vortex Lattices in Neutron Interferometry
    DOI 10.48550/arxiv.2205.00536
    Type Preprint
    Author Geerits N
    Link Publication
  • 2021
    Title Time-of-flight modulated intensity small-angle neutron scattering measurement of the self-diffusion constant of water
    DOI 10.1107/s1600576721002612
    Type Journal Article
    Author Kuhn S
    Journal Journal of Applied Crystallography
    Pages 751-758
    Link Publication

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